The Resource Selectivity in the synthesis of cyclic sulfonamides : application in the synthesis of natural products, Kimberly Geoghegan

Selectivity in the synthesis of cyclic sulfonamides : application in the synthesis of natural products, Kimberly Geoghegan

Label
Selectivity in the synthesis of cyclic sulfonamides : application in the synthesis of natural products
Title
Selectivity in the synthesis of cyclic sulfonamides
Title remainder
application in the synthesis of natural products
Statement of responsibility
Kimberly Geoghegan
Creator
Author
Subject
Genre
Language
eng
Summary
In the area of organic chemistry one major challenge we are currently faced with is how to assemble potentially useful molecules in new ways that generate molecular complexity and in sequences that are as efficient as possible. Our efforts in this regard, specifically for the preparation of amino containing compounds incorporating an aromatic ring, are described in this doctoral thesis. We discovered an interesting regioselectivity in an intramolecular Heck reaction, which we studied for a series of substrates that are unbiased in terms of the size of the newly formed ring, where very high levels of selectivity in relation to the new carbon-carbon bond are typically observed. DFT calculations were performed to attempt to shed light on the reaction sequence. This regioselective Heck reaction, combined with the reductive removal of the temporary amino-protecting group, allowed us to synthesize the Sceletium alkaloids: mesembrane, mesembranol and mesembrine
Member of
Cataloging source
GW5XE
http://library.link/vocab/creatorName
Geoghegan, Kimberly
Dewey number
547/.4
Illustrations
illustrations
Index
no index present
LC call number
RM666.S88
Literary form
non fiction
Nature of contents
  • dictionaries
  • bibliography
Series statement
Springer Theses,
http://library.link/vocab/subjectName
  • Sulfonamides
  • SCIENCE
Label
Selectivity in the synthesis of cyclic sulfonamides : application in the synthesis of natural products, Kimberly Geoghegan
Link
https://ezproxy.lib.ou.edu/login?url=http://link.springer.com/10.1007/978-3-319-10338-9
Instantiates
Publication
Note
"Doctoral thesis accepted by the University College Dublin, Ireland."
Antecedent source
unknown
Bibliography note
Includes bibliographical references
Carrier category
online resource
Carrier category code
cr
Carrier MARC source
rdacarrier
Color
multicolored
Content category
text
Content type code
txt
Content type MARC source
rdacontent
Dimensions
unknown
Extent
1 online resource (xiii, 151 pages)
File format
unknown
Form of item
online
Isbn
9783319103372
Level of compression
unknown
Media category
computer
Media MARC source
rdamedia
Media type code
c
Note
SpringerLink
Other control number
10.1007/978-3-319-10338-9
Other physical details
illustrations (some color).
Quality assurance targets
not applicable
Reformatting quality
unknown
Sound
unknown sound
Specific material designation
remote
System control number
  • (OCoLC)889945713
  • (OCoLC)ocn889945713
Label
Selectivity in the synthesis of cyclic sulfonamides : application in the synthesis of natural products, Kimberly Geoghegan
Link
https://ezproxy.lib.ou.edu/login?url=http://link.springer.com/10.1007/978-3-319-10338-9
Publication
Note
"Doctoral thesis accepted by the University College Dublin, Ireland."
Antecedent source
unknown
Bibliography note
Includes bibliographical references
Carrier category
online resource
Carrier category code
cr
Carrier MARC source
rdacarrier
Color
multicolored
Content category
text
Content type code
txt
Content type MARC source
rdacontent
Dimensions
unknown
Extent
1 online resource (xiii, 151 pages)
File format
unknown
Form of item
online
Isbn
9783319103372
Level of compression
unknown
Media category
computer
Media MARC source
rdamedia
Media type code
c
Note
SpringerLink
Other control number
10.1007/978-3-319-10338-9
Other physical details
illustrations (some color).
Quality assurance targets
not applicable
Reformatting quality
unknown
Sound
unknown sound
Specific material designation
remote
System control number
  • (OCoLC)889945713
  • (OCoLC)ocn889945713

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