The Resource Read-out and coherent manipulation of an isolated nuclear spin : using a single-molecule magnet spin-transistor, Stefan Thiele

Read-out and coherent manipulation of an isolated nuclear spin : using a single-molecule magnet spin-transistor, Stefan Thiele

Label
Read-out and coherent manipulation of an isolated nuclear spin : using a single-molecule magnet spin-transistor
Title
Read-out and coherent manipulation of an isolated nuclear spin
Title remainder
using a single-molecule magnet spin-transistor
Statement of responsibility
Stefan Thiele
Creator
Author
Subject
Genre
Language
eng
Summary
This thesis sheds new light on the worldwide first electrical manipulation of a single nuclear spin. Over the last four decades, the size of a bit, the smallest logical unit in a computer, has decreased by more than two orders of magnitude and will soon reach a limit where quantum phenomena become important. Inspired by the power of quantum mechanics, researchers have already identified pure quantum systems, having, analog to a classical bit, two controllable and readable states. In this regard, the inherent spin of electrons or nuclei with its two eigenstates, spin up and spin down, is a promising candidate. Using expertise in the field of single-molecule magnets, the author developed a molecular transistor, which allows quantum information to be written onto a single nuclear spin by means of an electric field only, and, in addition, enables the electronic read-out of this quantum state. This novel approach opens a path to addressing and manipulating individual nuclear spins within a very confined space (a single molecule), at high speed. Thus, the author was able to show that single molecule magnets are promising candidates for quantum information processing, which is triggering a new field of research towards molecular quantum electronics
Member of
Cataloging source
N$T
http://library.link/vocab/creatorName
Thiele, Stefan
Dewey number
539.725
Index
no index present
LC call number
QC793.3.S6
Literary form
non fiction
Nature of contents
  • dictionaries
  • bibliography
Series statement
Springer theses
http://library.link/vocab/subjectName
  • Nuclear spin
  • SCIENCE
  • Nuclear spin
  • Physics
  • Quantum Information Technology, Spintronics
  • Biological and Medical Physics, Biophysics
  • Nuclear Physics, Heavy Ions, Hadrons
  • Magnetism, Magnetic Materials
  • Biophysics
  • Atomic & molecular physics
  • Electricity, electromagnetism & magnetism
  • Quantum physics (quantum mechanics & quantum field theory)
Label
Read-out and coherent manipulation of an isolated nuclear spin : using a single-molecule magnet spin-transistor, Stefan Thiele
Link
https://ezproxy.lib.ou.edu/login?url=http://link.springer.com/10.1007/978-3-319-24058-9
Instantiates
Publication
Copyright
Note
"Doctoral thesis accepted by the University of Grenoble, France."
Antecedent source
unknown
Bibliography note
Includes bibliographical references
Carrier category
online resource
Carrier category code
cr
Carrier MARC source
rdacarrier
Color
multicolored
Content category
text
Content type code
txt
Content type MARC source
rdacontent
Contents
  • Supervisor's Foreword; Abstract; Acknowledgements; Contents; 1 Introduction; 1.1 Molecular Spintronics; 1.2 Quantum Information Processing; 1.3 Thesis Outline; References; 2 Single Electron Transistor; 2.1 Equivalent Circuit; 2.2 Coulomb Blockade; 2.3 Cotunneling Effect; 2.4 Kondo Effect; References; 3 Magnetic Properties of TbPc2; 3.1 Structure of TbPc2; 3.2 Electronic Configuration of Tb3+; 3.3 Zeeman Effect; 3.4 Electron-Electron Interaction; 3.5 Spin-Orbit Interaction; 3.6 Ligand-Field Interaction; 3.7 Hyperfine Interaction; 3.8 Magnetization Reversal
  • 3.8.1 Quantum Tunneling of Magnetization3.8.2 Direct Transtions; References; 4 Experimental Details; 4.1 Overview Setup; 4.2 Dilution Refrigerator; 4.3 3D Vector Magnet; 4.4 Current Leads; 4.5 Sample Holder; 4.6 Filter; 4.6.1 Low Frequency Filters; 4.6.2 High Frequency Filters; 4.7 Signal Transducer; 4.8 Real-Time Data Acquisition; 4.9 Sample Fabrication; 4.9.1 Nanowire Fabrication; 4.9.2 Electromigration; 4.9.3 Fabrication of a Molecular Spin Transistor; References; 5 Single-Molecule Magnet Spin-Transistor; 5.1 Mode of Operation; 5.2 Read-Out Quantum Dot
  • 5.3 Magneto-Conductance and Anisotropy5.4 Exchange Coupling; 5.5 2D Magneto-Conductance of the Read-Out Dot; 5.6 Electronic Spin Relaxation; 5.7 Quantum Tunneling of Magnetization; 5.8 Summary; References; 6 Nuclear Spin Dynamics -- T1; 6.1 Signal Analysis; 6.2 Relaxation Time T1 and Read-Out Fidelity F; 6.3 Quantum Monte Carlo Simulations; 6.3.1 Algorithm; 6.3.2 Including the Experimental Boundaries; 6.4 Comparison Experiment -- Simulation; 6.4.1 Relaxation Mechanism; 6.4.2 Dynamical Equilibrium; 6.4.3 Selection Rules; 6.5 Summary; References; 7 Nuclear Spin Dynamics -- Tast2; 7.1 Introduction
  • 7.1.1 Rabi Oscillations7.1.2 Hyperfine Stark Effect; 7.2 Coherent Nuclear Spin Rotations; 7.2.1 Frequency Calibration; 7.2.2 Rabi Oscillations; 7.3 Experimental Discussion of the Hyperfine Stark Effect; 7.3.1 DC Gate Voltage Induced Hyperfine Stark Effect; 7.3.2 AC Induced Hyperfine Stark Effect; 7.4 Theoretical Discussion of the Hyperfine Stark Effect; 7.5 Dephasing Time T*2; 7.5.1 Introduction; 7.5.2 Experimental Results; 7.5.3 Outlook; 7.6 Summary; References; 8 Conclusion and Outlook; References; Appendix ASpin; Appendix BStevens Operators; Appendix CQuantum Monte Carlo Code
Dimensions
unknown
Extent
1 online resource.
File format
unknown
Form of item
online
Isbn
9783319240589
Level of compression
unknown
Media category
computer
Media MARC source
rdamedia
Media type code
c
Note
SpringerLink
Other control number
10.1007/978-3-319-24058-9
Quality assurance targets
not applicable
Reformatting quality
unknown
Sound
unknown sound
Specific material designation
remote
System control number
  • (OCoLC)930703266
  • (OCoLC)ocn930703266
Label
Read-out and coherent manipulation of an isolated nuclear spin : using a single-molecule magnet spin-transistor, Stefan Thiele
Link
https://ezproxy.lib.ou.edu/login?url=http://link.springer.com/10.1007/978-3-319-24058-9
Publication
Copyright
Note
"Doctoral thesis accepted by the University of Grenoble, France."
Antecedent source
unknown
Bibliography note
Includes bibliographical references
Carrier category
online resource
Carrier category code
cr
Carrier MARC source
rdacarrier
Color
multicolored
Content category
text
Content type code
txt
Content type MARC source
rdacontent
Contents
  • Supervisor's Foreword; Abstract; Acknowledgements; Contents; 1 Introduction; 1.1 Molecular Spintronics; 1.2 Quantum Information Processing; 1.3 Thesis Outline; References; 2 Single Electron Transistor; 2.1 Equivalent Circuit; 2.2 Coulomb Blockade; 2.3 Cotunneling Effect; 2.4 Kondo Effect; References; 3 Magnetic Properties of TbPc2; 3.1 Structure of TbPc2; 3.2 Electronic Configuration of Tb3+; 3.3 Zeeman Effect; 3.4 Electron-Electron Interaction; 3.5 Spin-Orbit Interaction; 3.6 Ligand-Field Interaction; 3.7 Hyperfine Interaction; 3.8 Magnetization Reversal
  • 3.8.1 Quantum Tunneling of Magnetization3.8.2 Direct Transtions; References; 4 Experimental Details; 4.1 Overview Setup; 4.2 Dilution Refrigerator; 4.3 3D Vector Magnet; 4.4 Current Leads; 4.5 Sample Holder; 4.6 Filter; 4.6.1 Low Frequency Filters; 4.6.2 High Frequency Filters; 4.7 Signal Transducer; 4.8 Real-Time Data Acquisition; 4.9 Sample Fabrication; 4.9.1 Nanowire Fabrication; 4.9.2 Electromigration; 4.9.3 Fabrication of a Molecular Spin Transistor; References; 5 Single-Molecule Magnet Spin-Transistor; 5.1 Mode of Operation; 5.2 Read-Out Quantum Dot
  • 5.3 Magneto-Conductance and Anisotropy5.4 Exchange Coupling; 5.5 2D Magneto-Conductance of the Read-Out Dot; 5.6 Electronic Spin Relaxation; 5.7 Quantum Tunneling of Magnetization; 5.8 Summary; References; 6 Nuclear Spin Dynamics -- T1; 6.1 Signal Analysis; 6.2 Relaxation Time T1 and Read-Out Fidelity F; 6.3 Quantum Monte Carlo Simulations; 6.3.1 Algorithm; 6.3.2 Including the Experimental Boundaries; 6.4 Comparison Experiment -- Simulation; 6.4.1 Relaxation Mechanism; 6.4.2 Dynamical Equilibrium; 6.4.3 Selection Rules; 6.5 Summary; References; 7 Nuclear Spin Dynamics -- Tast2; 7.1 Introduction
  • 7.1.1 Rabi Oscillations7.1.2 Hyperfine Stark Effect; 7.2 Coherent Nuclear Spin Rotations; 7.2.1 Frequency Calibration; 7.2.2 Rabi Oscillations; 7.3 Experimental Discussion of the Hyperfine Stark Effect; 7.3.1 DC Gate Voltage Induced Hyperfine Stark Effect; 7.3.2 AC Induced Hyperfine Stark Effect; 7.4 Theoretical Discussion of the Hyperfine Stark Effect; 7.5 Dephasing Time T*2; 7.5.1 Introduction; 7.5.2 Experimental Results; 7.5.3 Outlook; 7.6 Summary; References; 8 Conclusion and Outlook; References; Appendix ASpin; Appendix BStevens Operators; Appendix CQuantum Monte Carlo Code
Dimensions
unknown
Extent
1 online resource.
File format
unknown
Form of item
online
Isbn
9783319240589
Level of compression
unknown
Media category
computer
Media MARC source
rdamedia
Media type code
c
Note
SpringerLink
Other control number
10.1007/978-3-319-24058-9
Quality assurance targets
not applicable
Reformatting quality
unknown
Sound
unknown sound
Specific material designation
remote
System control number
  • (OCoLC)930703266
  • (OCoLC)ocn930703266

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